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Angular distributions of single- and double-electron capture in very-slow Ar sup 6+ -Ar collisions

Conference ·
OSTI ID:6437489
; ; ; ; ; ; ;  [1]; ; ; ;  [2]
  1. Tennessee Univ., Knoxville, TN (USA). Dept. of Physics Oak Ridge National Lab., TN (USA)
  2. Manne Siegbahn Inst. of Physics, Stockholm (Sweden)
We have measured state-resolved angular distributions of one- and two-electron capture in 32 to 800 eV Ar{sup 6+} {minus} Ar collisions. The experimental energy-gain spectra show that single-electron capture mainly populates the 5s, 5p and 4f levels. We observe detailed structures in the corresponding angular distributions, but a final interpretation has to await a quantitative analysis of the collision dynamics. We tentatively ascribe the main features in the angular distribution of true double-electron capture at Q {approximately} 26 eV (4s4f and 4s5s) and Q {approximately} 42 eV (3d4d) to processes involving two consecutive one-electron transitions. For the transfer ionization process, we measure a Q-value of {approximately}eV, which we assign to autoionizing 4s5s (or 4s4f) levels. The 4s5s, 4s4f, and 3d4d levels all reside above the first ionization limit of Ar{sup 4+}, but we find that the 3d4d level stabilizes through radiative decay. 8 refs., 4 figs.
Research Organization:
Oak Ridge National Lab., TN (USA)
Sponsoring Organization:
DOE/ER; NSF; SENSRC
DOE Contract Number:
AC05-84OR21400
OSTI ID:
6437489
Report Number(s):
CONF-901116-13; ON: DE91001217
Country of Publication:
United States
Language:
English