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Graphite aluminum- and silicon carbide-coated current collectors for sodium-sulfur cells

Journal Article · · J. Electrochem. Soc.; (United States)
DOI:https://doi.org/10.1149/1.2114096· OSTI ID:6401347

The electrical performance and corrosion of current collectors made from graphite foil bonded to aluminum and from stainless steel protected by silicon carbide coating are compared to current collectors protected by chromium coatings. The testing is done in corrosion cells operated under dynamic conditions in Na/sub 2/S/sub 5/ melt at 350/sup 0/C. The cells are operated under both cathodic and anodic potentials of 100-300 mV measured with respect to carbon reference electrodes. The current collectors made from graphite foil, 127 ..mu..m thick, bonded to aluminum have lowest total impedances (ohmic plus polarization) of 2.0 and 5.4 ..cap omega..-cm/sup 2/ under cathodic and anodic potential of 300 mV. The corresponding values for silicon carbide coatings, 1.8-2.0 ..mu..m thick, are 2.9 and 19.0 ..cap omega..-cm/sup 2/, and, for chromium coating about50 ..mu..m thick, 3.2 and 10.7 ..cap omega..-cm/sup 2/. No, or very little, corrosion is observed on the graphite/aluminum samples or on the silicon carbide-coated samples over a period of 2-3 months.

Research Organization:
Ford Motor Company, Dearborn, Michigan
OSTI ID:
6401347
Journal Information:
J. Electrochem. Soc.; (United States), Journal Name: J. Electrochem. Soc.; (United States) Vol. 132:5; ISSN JESOA
Country of Publication:
United States
Language:
English