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Nitrogen oxide formation from Australian coals

Journal Article · · Combust. Flame; (United States)

The evolution of fuel nitrogen during devolatilization and the formation of NO/sub x/ during combustion were studied for two Australian coals in crucible, thermobalance, and rapid heating (drop-tube furnace) experiments. The evolution of coal nitrogen during devolatilization was dependent on both temperature and mode of heating. Under near stoichiometric combustion, 20-30% of coal nitrogen was converted to NO/sub x/. Conversion increased markedly with increased fuel-lean conditions. The NO/sub x/ formed from volatiles was proportional to the fraction of coal nitrogen evolved as HCN and NH3. The combustion of char at various temperatures and stoichiometries showed that the conversion of char nitrogen to NO/sub x/ depended primarily on char burnout. The contribution of char nitrogen to NO/sub x/ formation was greater than that of volatile nitrogen under fuel-rich conditions.

OSTI ID:
6320989
Journal Information:
Combust. Flame; (United States), Journal Name: Combust. Flame; (United States) Vol. 62:1; ISSN CBFMA
Country of Publication:
United States
Language:
English