Suppression of charge scattering in Moessbauer experiments using synchrotron radiation

Conference · Wed Jan 01 04:00:00 EST 1992

OSTI ID:6277143

Bergmann, U; Siddons, D P; Hastings, J B

The extremely small ratio of linewidth to energy combined with the character of recoil free absorption and reemission makes the low lying nuclear resonances a unique spectroscopic tool. Further, considering the simplicity of performing Moessbauer experiments, they have become very useful in a wide range of disciplines. [sup 57]Fe has remained the most widely used isotope despite its low natural abundance (2%) because iron is ubiquitous in nature and shows a strong effect. The energy width of this resonance corresponds to a lifetime of 140 nsec of the excited state. Therefore in principle time differential spectroscopy is possible. Using the time differential measurement one is no longer restricted to a nuclear source, in fact a short pulse excitation is favored in such experiments. The concept of using a pulsed source and time gating to isolate the resonant scattering was already suggested in 1962. In 1974 it was noted that synchrotron radiation (SR) was ideally suited to this task. Although the time gating technique is conceptually simple the bandwidth of SR poses significant technical difficulties. In this paper we will discuss the extraction of the nuclear signal from the overwhelming background, which is the central problem in SR-based Moessbauer experiments. We will only, consider the [sup 57]Fe-isotope, although other isotopes might be of interest in a SR-based experiment. Although SR sources have the disadvantages of creating this high background and being limited in beam-time and location, new and unique opportunities make them very attractive even with these difficulties. For this reason research and development groups at every major SR facility worldwide are increasingly working on Moessbauer experiments, stimulated by the first successful observation of nuclear Bragg scattering (NBS) using SR in 1984.

• Research Organization: Brookhaven National Lab., Upton, NY (United States)
• Sponsoring Organization: DOE; USDOE, Washington, DC (United States)
• DOE Contract Number: AC02-76CH00016
• OSTI ID: 6277143
• Report Number(s): BNL-48963; CONF-9208186--4; ON: DE93015406
• Country of Publication: United States
• Language: English

Related Subjects

36 MATERIALS SCIENCE
360104 -- Metals & Alloys-- Physical Properties
665100* -- Nuclear Techniques in Condensed Matter Physics -- (1992-)
75 CONDENSED MATTER PHYSICS
SUPERCONDUCTIVITY AND SUPERFLUIDITY
BRAGG REFLECTION
BREMSSTRAHLUNG
COHERENT SCATTERING
DIFFRACTION
ELECTROMAGNETIC RADIATION
EVEN-ODD NUCLEI
FILMS
INELASTIC SCATTERING
INTERMEDIATE MASS NUCLEI
IRON 57
IRON ISOTOPES
ISOTOPES
MOESSBAUER EFFECT
NUCLEI
RADIATIONS
REFLECTION
RESONANCE SCATTERING
SCATTERING
STABLE ISOTOPES
SYNCHROTRON RADIATION
THIN FILMS
TIME DEPENDENCE
X-RAY DIFFRACTION