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Absolute-cross-section measurements for electron-impact ionization of triply charged inert-gas ions: Ne/sup 3 +/, Ar/sup 3 +/, Kr/sup 3 +/, and Xe/sup 3 +/

Journal Article · · Phys. Rev. A; (United States)
Electron-ion crossed beams have been employed to obtain absolute cross sections for single ionization of Ne/sup 3 +/, Ar/sup 3 +/, Kr/sup 3 +/, and Xe/sup 3 +/. These data reveal a steady progression from excellent agreement with theory and semiempirical formulas for Ne/sup 3 +/ to significant departures from any simple models for Xe/sup 3 +/. For Ar/sup 3 +/ some small departure from the models is apparent and the measurements agree with previous experimental results of Mueller et al. For Kr/sup 3 +/ and Xe/sup 3 +/ the measured cross sections in the energy range below four threshold units exhibit complex structure and exceed estimates of direct ionization by roughly factors of 2 and 3, respectively. These features are attributed to indirect ionization processes involving excitation of inner-shell electrons, and the observed cross-section shapes imply that the excitation-autoionization features cannot be simply attributed to dipole-allowed excitation transitions. Ionization rates for Maxwellian electron-temperature distributions are calculated from the data.
Research Organization:
Physics Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37830
DOE Contract Number:
W-7405-ENG-26
OSTI ID:
6266464
Journal Information:
Phys. Rev. A; (United States), Journal Name: Phys. Rev. A; (United States) Vol. 27:2; ISSN PLRAA
Country of Publication:
United States
Language:
English