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Free jet cooled laser-induced fluorescence spectrum of methoxy. 1. Vibronic analysis of the /tilde A/ and /tilde X/ states

Journal Article · · J. Phys. Chem.; (United States)
DOI:https://doi.org/10.1021/j100332a014· OSTI ID:6255318
The methoxy free radical has been formed in a supersonic free jet expansion by KrF photolysis of methyl nitrite. Its laser-induced fluorescence excitation and wavelength-resolved emission spectra have been recorded at low temperature. This paper reports the vibronic analysis of the CH/sub 3/O and CD/sub 3/O /tilde A//sup 2/A/sub 1/ /leftrightarrow/ /tilde X//sup 2/E electronic spectra. A new value for the electronic origin has been determined as well as a nearly complete set of vibrational frequencies.
Research Organization:
Ohio State Univ., Columbus (USA)
OSTI ID:
6255318
Journal Information:
J. Phys. Chem.; (United States), Journal Name: J. Phys. Chem.; (United States) Vol. 92:21; ISSN JPCHA
Country of Publication:
United States
Language:
English