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Nitrogen compounds in Colorado shale oils

Journal Article · · Am. Chem. Soc., Div. Pet. Chem., Prepr.; (United States)
OSTI ID:6219261

The nitrogen contents of Colorado shale oils, produced in internally fired retorts, approximate 2% by weight for the oils that have been investigated. The quantity of nitrogen in the oils depends on the conditions in the retort producing the oil. About 2/3 of the nitrogen compounds in the naphtha are pyridines. The other 1/3 is predicted to be C-alkylated pyrroles. A naphtha, produced by destructive hydrogenation of a crude shale oil, contained both pyridines and anilines. A heavy gas-oil fraction consisted of 40% nitrogen compounds. These were one-, two-, and multi-ring compounds. For the multi-ring compounds, the data suggest more than one heteroatom per molecule. Porphyrins are shown to be present in shale oil and to be changed from those present in the oil shale. Groennings' extraction is a satisfactory method for concentration of the porphyrins.

Research Organization:
Wyoming Univ.
OSTI ID:
6219261
Journal Information:
Am. Chem. Soc., Div. Pet. Chem., Prepr.; (United States), Journal Name: Am. Chem. Soc., Div. Pet. Chem., Prepr.; (United States) Vol. 10:2; ISSN ACPCA
Country of Publication:
United States
Language:
English