Skip to main content
U.S. Department of Energy
Office of Scientific and Technical Information

Use of resonance epithermal neutron scattering for the study of condensed matter

Thesis/Dissertation ·
OSTI ID:6181948

Resonant epithermal neutron scattering studies provide a new regime for the study of the properties of condensed matter. The differenital scattering cross section is developed in a resonant correlation function formalism involving the positions of two scattering centers at four different times. The resonant correlation functions contain information which cannot be obtained from a study of the Van Hove correlation functions for thermal neutron scattering, and these resonant correlation functions enable one to observe phenomena which are beyond neutron scattering. It is shown that the lowest order correction to the short collision time limit yields a force density correlation function. Resonant neutron scattering provides a means of determining the amplitudes of specific anharmonic phonon interactions of cubic order. When this method is turned to the study of diffusion, one obtains higher order diffusive propagators which give the conditional probabilities for diffusion over two distinct intervals of time. The resonant selection of virtual excited states enables one to observe the diffusion of molecules in definite states of vibrational excitation.

OSTI ID:
6181948
Country of Publication:
United States
Language:
English