Skip to main content
U.S. Department of Energy
Office of Scientific and Technical Information

Neutronic analysis of critical configurations in geologic repositories. 2: Highly enriched uranium

Journal Article · · Nuclear Science and Engineering
OSTI ID:616413
;  [1]
  1. Univ. of California, Berkeley, CA (United States). Dept. of Nuclear Engineering
Neutronic characteristics are investigated of critical configurations consisting of U and moist rock, which may be formed if large enough quantities of highly enriched U (HEU) are released, transported, and deposited in the rock below the repository. A companion study investigated neutronic characteristics of similar critical configurations consisting of weapons-grade Pu (wPu) and moist rock. Two modes of U deposition are considered: uniform homogeneous and heterogeneous. The latter is assumed to be of the form of thin planar deposition layers separated by relatively thick slabs of rock, making a constant pitch lattice. Three neutronic characteristics are examined: the critical U loading, and the variation, with the change of operating conditions, of the multiplication factor k; the time-eigenvalue a; and the effective neutron generation time {Lambda}. They are compared against the characteristics of the corresponding wPu-rock systems. The study is done parametrically by solving time-independent transport equations. The effect of various mechanisms (including water removal, U and rock temperature increase, homogenization of fissile and rock materials, and the system expansion) on the neutronic characteristics is studied independently. A surprising finding is that heterogeneous depositions of HEU in moist rock can have a positive reactivity feedback due to spectrum hardening. Moreover, the magnitude and temperature dependence of heterogeneous U-rock systems can be comparable to those of Pu-rock systems despite the fact that they are due to entirely different mechanisms. It is concluded that heterogeneous HEU deposits in moist rock can be just about as autocatalytic as critical wPu deposits but require approximately twice the critical mass.
Sponsoring Organization:
Los Alamos National Lab., NM (United States)
OSTI ID:
616413
Journal Information:
Nuclear Science and Engineering, Journal Name: Nuclear Science and Engineering Journal Issue: 1 Vol. 129; ISSN NSENAO; ISSN 0029-5639
Country of Publication:
United States
Language:
English

Similar Records

Considerations of autocatalytic criticality of fissile materials in geologic repositories
Journal Article · Sun Sep 01 00:00:00 EDT 1996 · Nuclear Technology · OSTI ID:379832

Neutronic analysis of critical configurations in geologic repositories. 1: Weapons-grade plutonium
Journal Article · Fri Oct 31 23:00:00 EST 1997 · Nuclear Science and Engineering · OSTI ID:556638

External Criticality Risk of Immobilized Plutonium Waste Form in a Geologic Repository
Technical Report · Sun Mar 11 19:00:00 EST 2001 · OSTI ID:837027