Skip to main content
U.S. Department of Energy
Office of Scientific and Technical Information

The roles of amorphous grain boundaries and the {beta}-{alpha} transformation in toughening SiC

Journal Article · · Acta Materialia
;  [1];  [2]
  1. Lawrence Berkeley National Lab., CA (United States). Center for Advanced Materials
  2. Univ. of California, Berkeley, CA (United States). Dept. of Materials Science and Mineral Engineering

Controlled development of the ceramic microstructure has produced silicon carbide (SiC) with a toughness three times that of a commercial SiC, Hexoloy-SA, coupled with > 50% improvement in strength. Al, B and C were used as sintering additives, hence the designation ABC-SiC. These additives facilitated full densification at temperature as low as 1,700 C, the formation of an amorphous phase at the grain boundaries to enhance intergranular fracture, and the promotion of an elongated microstructure to enhance crack deflection and crack bridging. Comparisons of microstructures and fracture properties have been made between the present ABC-SiC, Hexoloy-SA and other reported SiC ceramics sintered with YAG or Al{sub 2}O{sub 3}. The Al-O chemistry of the amorphous phase in the ABC-SiC accounted for the intergranular fracture vs the transgranular fracture in Hexoloy-SA. An interlocking plate-like grain structure developed during the {beta} to {alpha} transformation without limiting densification. The combined microstructural developments improved both strength and toughness.

Sponsoring Organization:
USDOE, Washington, DC (United States)
DOE Contract Number:
AC03-76SF00098
OSTI ID:
616390
Journal Information:
Acta Materialia, Journal Name: Acta Materialia Journal Issue: 5 Vol. 46; ISSN 1359-6454; ISSN ACMAFD
Country of Publication:
United States
Language:
English

Similar Records

Microstructural development to toughen SiC
Conference · Mon Dec 30 23:00:00 EST 1996 · OSTI ID:470915

In situ toughened SiC ceramics with Al-B-C additions and oxide-coated SiC platelet/SiC composites
Technical Report · Sat Nov 30 23:00:00 EST 1996 · OSTI ID:414374

Crack-growth resistance-curve behavior in silicon carbide: Small versus long cracks
Journal Article · Mon Sep 01 00:00:00 EDT 1997 · Journal of the American Ceramic Society · OSTI ID:554014