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Observations of tropospheric trace gases and techniques for assessing the regional transport of air pollutants

Thesis/Dissertation ·
OSTI ID:6154498
Two techniques were used to assess regional transport of gaseous air pollutants. The first involved conducting airborne measurements of vertical profiles of the trace gases CO, O/sub 3/, and reactive nitrogen compounds near convective clouds, followed by analysis and interpretation with detailed meteorological data. The second technique involved applying spectral and cross spectral analyzes to surface-based time series of simultaneous trace gas concentrations and wind data. Airborne measurements were conducted near a line of deep convective clouds in south-central Oklahoma. Trace gas concentrations in the upper tropospheric outflow region of these clouds were near levels found in the surrounding environment. Meteorological analyses showed that these clouds were located above a cold front, which prevented the entry of air from the boundary layer directly below the cloud. These results suggest that the large amount of vertical trace gas transport noted in previous observations and model results cannot simply be extrapolated to all convective cells.
Research Organization:
Maryland Univ., College Park (USA)
OSTI ID:
6154498
Country of Publication:
United States
Language:
English