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Natural radioactivity due to RaDEF and beryllium-7 in the environment

Thesis/Dissertation ·
OSTI ID:6138863
Sharp increases in the /sup 210/Po//sup 210/Pb activity ratios were observed during the year 1981, one year after Mount St. Helens erupted on May 18, 1980. However, individual /sup 210/Pb and /sup 210/Po concentrations and fallout profiles did not alter markedly before or after this volcanic event. Bimonthly average /sup 210/Po//sup 210/Pb activity ratio of 0.77 was observed for the months of January-February, 1981. Results obtained from our data for 134 samples of rain and snow analyzed for /sup 210/Pb and /sup 210/Po between November 1, 1979, and December 31, 1981, show that the high /sup 210/Pb activity ratios were accompanied by high /sup 7/Be//sup 210/Pb and /sup 90/Sr//sup 210/Pb ratios for the same period indicating a stratospheric fallout. Infinity values obtained for aerosol residence times may have been the result of ash and fine debris enrichment of the stratosphere, and not due to any /sup 210/Po excess. /sup 210/Pb and /sup 210/Po flux from the Fayetteville soil samples being negligible, soil entrainment of the sampling site seems to be minimal. The concentrations of /sup 7/Be and /sup 210/Pb (RaD) were measured in sequentially sampled rainstorm of March 15, 1982, that occurred over Fayetteville (36/sup 0/N, 94/sup 0/W), Arkansas. /sup 7/Be//sup 210/Pb ratios ranged from 1.8 to 16.7 (Ci/Ci) and covered the entire range of values observed for individual samples of rain and snow (Ali Saleh, 1983). Two air-masses may have dominated the Northwest Arkansas region temporarily during this period.
Research Organization:
Arkansas Univ., Fayetteville (USA)
OSTI ID:
6138863
Country of Publication:
United States
Language:
English