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Title: Total neutron cross sections of berkelium-249 and californium-249 below 100 eV

Technical Report ·
OSTI ID:6123615

The neutron total cross sections of /sup 249/Bk and /sup 249/Cf have been measured from 0.03 to 100 eV using the Oak Ridge Electron Linear Accelerator (ORELA) as a source of pulsed neutrons. The 1.6 mm dia. cylindrical transmission samples contained initially up to 5.3 mg of 98% /sup 249/Bk and 2% /sup 249/Cf: 4.5 years later, when the final measurements were made, the composition of the samples had become 2.5% /sup 249/Bk, 96.9% /sup 249/Cf, and 0.6% /sup 245/Cm. Samples were cooled with liquid nitrogen to reduce Doppler broadening. Thirty-nine resonances were identified in /sup 249/Bk and analyzed using a single-level Breit-Wigner formalism. Fifty-five resonances were identified in /sup 249/Cf and analyzed using an R-matrix multilevel formalism. Fifty-five resonances were identified in /sup 249/Cf and analyzed using an R-matrix multilevel formalism. The resonance parameters obtained have been used to determine the average level spacings and the s-wave neutron and fission strength functions. Where possible, bound-level parameters were derived to fit the thermal neutron total cross section data.

Research Organization:
Du Pont de Nemours (E.I.) and Co., Aiken, SC (USA). Savannah River Lab.; Oak Ridge National Lab., TN (USA)
DOE Contract Number:
AC09-76SR00001
OSTI ID:
6123615
Report Number(s):
DP-MS-83-10; ON: DE83013681
Country of Publication:
United States
Language:
English