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Microwave sintered silicon nitride ceramics

Conference ·
OSTI ID:6077408

Silicon nitride-based materials are processed using a variety of thermal heating techniques and procedures, such as sintering, reaction-bonding, and annealing. For sintering, typical silicon nitride processing starts with high {alpha}-phase Si{sub 3}N{sub 4} powders mixed with sintering aids, such as MgO, Y{sub 2}O{sub 3}, and Al{sub 2}O{sub 3}. After consolidation of the mixtures into a shape, they are heated in a nitrogen atmosphere to temperatures of 1700 to 1900{degrees}C to densify. The sintering temperature is dependent on the type and quantity of sintering additives utilized. Densification of silicon nitride compacts occurs through a number of distinct steps. Microwave heating has the capability for volumetric thermal heating of ceramic materials. Silicon nitride-based materials heat in a microwave field by coupling to the sintering additives or grain boundary phases. Previous studies on microwave processing of silicon nitride have reported improved densification during sintering, accelerated nitridation of silicon, and improved high-temperature mechanical properties with thermal annealing of dense materials. In the present research, microwave-sintered silicon nitride ceramics were examined, and the densification behavior and microstructure development correlated with the mechanical properties.

Research Organization:
Oak Ridge National Lab., TN (United States)
Sponsoring Organization:
DOE; USDOE, Washington, DC (United States)
DOE Contract Number:
AC05-84OR21400
OSTI ID:
6077408
Report Number(s):
CONF-910908-2; ON: DE92004405
Country of Publication:
United States
Language:
English