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Dependence of the electronic effects of substituents in. pi. systems on the character of the. pi. -molecular orbitals. VIII. The parametrization of simple molecular-orbital calculations of the effect of substituents on the energies of the. pi. levels in aromatic molecules

Journal Article · · J. Org. Chem. USSR (Engl. Transl.); (United States)
OSTI ID:6036292
For the case of calculations on the vertical ionization potentials of di- and poly-substituted benzenes, monosubstituted pyridines, naphthalenes, and anthracenes it was shown that the approximation based on the linear combination of the occupied orbitals of the parent molecules and substituents makes it possible to estimate fairly well the change in the energies of the two highest occupied ..pi.. levels of the aromatic molecules under the influence of the substituents by means of the parameters determined from the ionization potentials of monosubstituted benzenes (I/sub calc/ = 0.97 x I/sub expt/ + 0.32; n = 191, r = 0.992, s = 0.11).
Research Organization:
Novosibirsk Institute of Organic Chemistry, USSR
OSTI ID:
6036292
Journal Information:
J. Org. Chem. USSR (Engl. Transl.); (United States), Journal Name: J. Org. Chem. USSR (Engl. Transl.); (United States) Vol. 22:6; ISSN JOCYA
Country of Publication:
United States
Language:
English

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