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U.S. Department of Energy
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Microcellular polymer foams prepared by thermally-induced phase separation

Conference ·
OSTI ID:5952184

Thermally-induced phase separation (TIPS) of polymer solutions is discussed. The process consists of three steps. In the first step, a polymer and solvent are heated above their critical temperature to achieve a homogeneous polymer solution. Next, the solution is quenched in a controlled fashion in order to initiate thermally- induced phase separation, TIPS. Under some circumstances, TIPS can result in the formation of bi-continuous phases, a polymer-rich phase and a solvent-rich phase. Once phase separation has occurred, the solution can be frozen which effectively terminates phase separation. Alternatively with semi-crystalline polymers the solution may form a stable gel after TIPS. In the final step, the solvent is removed by sublimation of the frozen solvent or by liquid extraction of a resulting gel leaving behind a microcellular polymer foam. By controlling the phase separation during the quench, the foam morphology, foam density, and cell size can be varied. 3 refs., 3 figs.

Research Organization:
Sandia National Labs., Albuquerque, NM (USA)
DOE Contract Number:
AC04-76DP00789
OSTI ID:
5952184
Report Number(s):
SAND-89-1060C; CONF-8907112-1; ON: DE89015490
Country of Publication:
United States
Language:
English