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Calculations for isotopically tailored ceramics in fission and fusion reactors

Journal Article · · Advanced Ceramic Materials; (USA)
Ceramics in the 14-MeV neutron environment of a fusion reactor will experience irradiation effects not only from displacement events but also from accumulation of the transmutation gases He and H. Combined damage effects from these sources can be approximated by irradiation testing of isotopically tailored ceramics in a mixed-spectrum fission reactor, where fast neutrons will produce the displacements and thermal neutrons will induce the gas-producing reactions {sup 17}O(n,{alpha}){sup 14}C and {sup 14}N(n,p){sup 14}C. To aid in the design of such an experiment, calculations have been made to determine the amount of the isotopes {sup 17}O and {sup 15}N (the latter to reduce excess production of H) needed in the test ceramic Si{sub 3}Al{sub 3}O{sub 3}N{sub 5} and {sup 17}O (for generation of He only) needed in Al{sub 2}O{sub 3}. Reference irradiation sources were the STARFIRE fusion reactor and the HFIR fission reactor. Results indicate that the desired ratios of gas to displacement energy can be obtained by incorporating 57% {sup 17}O and 90.6% {sup 15}N into sialon, and 17.9% {sup 17}O into alumina.
OSTI ID:
5924095
Journal Information:
Advanced Ceramic Materials; (USA), Journal Name: Advanced Ceramic Materials; (USA) Vol. 3:4; ISSN 0883-5551; ISSN ACEME
Country of Publication:
United States
Language:
English