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Increased flux pinning upon thermal-neutron irradiation of uranium-doped YBa/sub 2/Cu/sub 3/O/sub 7/

Journal Article · · Phys. Rev. B: Condens. Matter; (United States)
To assess fission-fragment damage as flux-pinning centers, sintered compacts of YBa/sub 2/Cu/sub 3/O/sub 7/ were prepared with uranium additions of 150 and 380 atomic ppm and exposed to thermal neutron fluences of 4.3/times/10/sup 17/, 1.2/times/10/sup 18/, and 4.0/times/10/sup 18//cm/sup 2/. Magnetic hysteresis measurements were made as functions of temperature at fields up to 2.5 T. The hysteresis at 1 T for the sample containing 150 ppm uranium increased upon an irradiation of 1.2/times/10/sup 18//cm/sup 2/ by 3.7 times at 4.5 K, 20 times at 63 K, and 8.3 times at 77 K. Much smaller increases in magnetic hysteresis were observed in undoped samples exposed to thermal neutrons. Critical-current densities were calculated from the hysteresis observed at 1 T using the critical-state model, assuming the currents to be restricted to the grains (/approx/5 /mu/m radius). For the 150 ppm, 1.2/times/10/sup 18//cm/sup 2/ sample, the 1-T intragranular critical-current densities obtained are 1.5/times/10/sup 7/, 1.0/times/10/sup 6/, and 1.4/times/10/sup 5/ A/cm/sup 2/ at temperatures of 4.5, 63, and 77 K, respectively. The critical temperatures by an ac susceptibility technique showed that the 4/times/10/sup 18//cm/sup 2/ irradiation lowered the onset critical temperatures only slightly, from 91 to 90 K and from 91.5 to 89 K for the 150 and 380 ppm samples, respectively.
Research Organization:
General Electric Research and Development, Schenectady, New York 12301 (US)
OSTI ID:
5917239
Journal Information:
Phys. Rev. B: Condens. Matter; (United States), Journal Name: Phys. Rev. B: Condens. Matter; (United States) Vol. 40:4; ISSN PRBMD
Country of Publication:
United States
Language:
English

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