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Compilation of criticality data involving thorium or 233U and light water moderation

Technical Report ·
DOI:https://doi.org/10.2172/5875312· OSTI ID:5875312
The literature has been searched for criticality data for light water moderated systems which contain thorium or /sup 233/U, and data found are compiled herein. They are from critical experiments, extrapolations, and exponential experiments performed with homogeneous solutions and metal spheres of /sup 233/U; with lattices of fuel rods containing highly enriched /sup 235/UO/sub 2/ - ThO/sub 2/ and /sup 233/UO/sub 2/ - ThO/sub 2/; and with arrays of cyclinders of /sup 233/U solutions. The extent of existing criticality data has been compared with that necessary to implement a thorium-based fuel cycle. No experiments have been performed with any solutions containing thorium. Neither do data exist for homogeneous /sup 233/U systems with H/U < 34, except for solid metal systems. Arrays of solution cylinders up to 3 x 3 x 3 have been studied. Data for solutions containing fixed or soluble poisons are very limited. All critical lattices using /sup 233/UO/sub 2/ - ThO/sub 2/ fuels (LWBR program) were zoned radially, and in most cases axially also. Only lattice experiments using /sup 235/UO/sub 2/ - ThO/sub 2/ fuels have been performed using a single fuel rod type. Critical lattices of /sup 235/UO/sub 2/ - ThO/sub 2/ rods poisoned with boron have been measured, but only exponential experiments have been performed using boron-poisoned lattices of /sup 233/UO/sub 2/ - ThO/sub 2/ rods. No criticality data exist for denatured fuels (containing significant amounts of /sup 238/U) in either solution or lattice configurations.
Research Organization:
Pacific Northwest Lab., Richland, WA (USA)
Sponsoring Organization:
USDOE National Nuclear Security Administration (NNSA), Nuclear Criticality Safety Program (NCSP)
DOE Contract Number:
AC06-76RL01830
OSTI ID:
5875312
Report Number(s):
PNL-2080-12
Country of Publication:
United States
Language:
English