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Nondestructive analysis of laser fusion microsphere targets using rotational Raman spectroscopy

Journal Article · · J. Appl. Phys.; (United States)
DOI:https://doi.org/10.1063/1.325981· OSTI ID:5859319
The use of rotational Raman scattering for nondestructive analysis of laser fusion microsphere targets is reported. Typical hollow-glass-microsphere sample characteristics are 100 ..mu..m in diameter, 1.0 ..mu..m in glass wall thickness, and 0.5 nl in volume, containing a mixture of hydrogen, deuterium, and tritium gases at pressures of 10--70 atm (total gas sample weights of 5 ng). Relative species mole fraction measurements for all hydrogen isotope species are determined from spectral peak height analysis of rotational Raman spectra. Accuracies of +- 0.01 (mole fraction) are obtained from spectra requiring 20 min scan time. Individual species detectability limits are less than 100 picogram. Absolute partial pressure measurements (accurate to +- 20%) are obtained using calibration spheres of known diameter and pressure.
Research Organization:
National Bureau of Standards, Washington, D.C. 20234
OSTI ID:
5859319
Journal Information:
J. Appl. Phys.; (United States), Journal Name: J. Appl. Phys.; (United States) Vol. 50:12; ISSN JAPIA
Country of Publication:
United States
Language:
English