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U.S. Department of Energy
Office of Scientific and Technical Information

Aerosol microphysics of indoor radon: Annual update, 1 October 1988--31 August 1989

Technical Report ·
OSTI ID:5837585
To provide an improved description for the deposition of charge on ultrafine aerosol particles, we have introduced for the first time into aerosol studies the ''jellium'' model potential to quantitatively describe the interaction energy at long range between a conducting particle and an ion (here modeled as a point charge). The benefit of utilizing this potential, in its linearized approximation, is that it accounts for the response of the particle's conduction electrons to the field of the ion rather than relying upon a macroscopic picture whose validity is nuclear for sufficiently small particles. In the limit of large separations or of larger particles, the jellium and image potentials converge rapidly implying that no inconsistency exists between the generally-accepted approach for larger particles and our contribution. As a part of our work, we have given an accurate fit to the experimental data in the literature on the charging rate of neutral particles in the 4--50 nm range of radii without the need for assumptions other than of the charging ion properties. The results of this work will contribute to the ability to model charged radon daughter cluster ion attachment to high-diffusivity particles and conversely to the ability to model charge attachment on high-diffusivity uncharged particles containing a radon daughter.
Research Organization:
Texas A and M Univ., College Station, TX (USA). Dept. of Nuclear Engineering
DOE Contract Number:
FG05-87ER60550
OSTI ID:
5837585
Report Number(s):
DOE/ER/60550-3; ON: DE89017359
Country of Publication:
United States
Language:
English