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Title: Improved multipass optics for diode laser spectroscopy

Journal Article · · Review of Scientific Instruments; (United States)
DOI:https://doi.org/10.1063/1.1144308· OSTI ID:5830316
; ; ;  [1]
  1. Molecular Sciences Research Center, Pacific Northwest Laboratory, Richland, Washington 99352 (United States)

Feedback between optical elements can be a major source of noise when trying to attain high sensitivity in infrared absorption experiments. We find that a conventional White-cell optical arrangement introduces etaloning fringes that modulate the peak-to-peak amplitude of our signals by 1 part in 16 666, a fractional change of 6[times]10[sup [minus]5]. Although relatively small, this noise'' is systematic and adds coherently with averaging, obscuring interesting absorption features. An easily constructed multipass optical system suited for performing high-resolution infrared spectroscopy in molecular beams is described. The design is based on a variation of the White cell and has been optimized for use with lead salt diode lasers. One of the key components in the improved design is the addition of an oscillating mirror for spoiling optical feedback generated by laser scatter and/or poor mode coupling of the laser to the multipass optics.

DOE Contract Number:
AC06-76RL01830
OSTI ID:
5830316
Journal Information:
Review of Scientific Instruments; (United States), Vol. 64:12; ISSN 0034-6748
Country of Publication:
United States
Language:
English