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Half-life of /sup 232/U

Journal Article · · Phys. Rev., C; (United States)
The half-life of /sup 232/U was determined by two independent methods: a specific activity method and a relative activity method involving the half-life of /sup 233/U. In the specific activity method, the ..cap alpha.. disintegration rate of /sup 232/U was determined by liquid scintillation counting as well as by ..cap alpha.. proportional counting, and the number of atoms of /sup 232/U was determined by isotope dilution mass spectrometry. The radiochemical purity of the purified /sup 232/U was confirmed by ..cap alpha.. spectrometry. A half-life value of 69.00 +- 0.40 yr was obtained. In the relative activity method, synthetic mixtures were prepared using isotopes of /sup 232/U and /sup 233/U. The ..cap alpha.. activity ratios in these mixtures were determined by ..cap alpha.. spectrometry and the atom ratios were obtained by mass spectrometry. The ..cap alpha.. activity ratios and the atom ratios were such that these could be measured with a high precision and accuracy. A half-life value of 68.81 +- 0.38 yr was obtained using the half-life of /sup 233/U as 1.592 x 10/sup 5/ yr. The average of these two independent determinations leads to a value of 68.90 +- 0.39 yr for the half-life of /sup 232/U. The uncertainty given on the values is a combination of the one standard deviation on the average value and the error evaluated from estimates on various error components. The values reported earlier are significantly higher as compared to the half-life value obtained in this work.
Research Organization:
Radiochemistry Division, Bhabha Atomic Research Centre, Trombay, Bombay 400 085, India
OSTI ID:
5812380
Journal Information:
Phys. Rev., C; (United States), Journal Name: Phys. Rev., C; (United States) Vol. 20:4; ISSN PRVCA
Country of Publication:
United States
Language:
English