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Synthesis and ESR investigation of new coordination compounds with a phenoxyl free radical ligand based on N-(3,5-DI-tert-butyl-2-hydroxyphenyl)salicylaldimine

Journal Article · · Journal of General Chemistry of the USSR (English Translation); (USA)
OSTI ID:5802083

A method is proposed for the preparation of 2-amino-4,6-di-tert-butylphenol. N-(3,5-Di-tert-butyl-2-hydroxyphenyl)salicylaldimine is readily mercurated with the formation of a mercury-containing free radical. Pd(II), Co(II), and VO(II) salicylaldiminates based on 2-amino-4,6-di-tert-butylphenol are capable of one-electron oxidation with the formation of metal-containing phenoxyl radicals. Analysis of the ESR spectra showed that the appearance of the metallocycle leads to a sharp increase in the stability of the radical system.

OSTI ID:
5802083
Journal Information:
Journal of General Chemistry of the USSR (English Translation); (USA), Journal Name: Journal of General Chemistry of the USSR (English Translation); (USA) Vol. 56:4; ISSN 0022-1279; ISSN JGCHA
Country of Publication:
United States
Language:
English

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