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Thermoluminescence systems with two or more glow peaks described by anomalous kinetic parameters

Conference ·
OSTI ID:5766286
The usual first and second order TL kinetic expressions are based on a number of assumptions, including the usually unstated assumption that charges released from one type of trap, giving rise to one glow peak, are not retrapped on other types of traps, associated with other glow peaks. Equations have been developed describing TL systems in which charges released from one type of trap may be retrapped in other types of traps. Called interactive kinetic equations, they are quite simple but have been studied by numerical methods. In particular, glow curves computed from the interactive kinetic equations have been regarded as data and analyzed by fitting them to the usual first and second order kinetic expressions. All of the anomalous features described above are reproduced. For example, usually the computed glow peaks are well fitted by the first and second order expressions over their upper 60 to 80% but not in the wings. This explains why the usual analysis methods, especially those utilizing peak temperature, full width, etc. appear to describe such peaks. Often unrealistic kinetic parameters are often obtained. Furthermore, the computed glow curves often reproduce the observed dependence on dose.
Research Organization:
Brookhaven National Lab., Upton, NY (USA)
DOE Contract Number:
AC02-76CH00016
OSTI ID:
5766286
Report Number(s):
BNL-33450; CONF-830573-6; ON: DE83016723
Country of Publication:
United States
Language:
English