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Nonsuperconducting phases at grain boundaries in YBa/sub 2/Cu/sub 3/O/sub x/ superconductors

Journal Article · · Int. J. Mod. Phys. B; (United States)
OSTI ID:5764009

The morphology, composition and phases of grain boundaries in YBa/sub 2/Cu/sub 3/O/sub x/ superconductors have been investigated by SEM, TEM and AES. The results show that some impure phase particles present at the grain boundary in the samples sintered at 940/sup 0/C for 26 hours, which grow to be a shell around the grain as the sintering temperature increases to 970/sup 0/C. No such particle has been found at the grain boundaries in the sample sintered at 920/sup 0/C for 26 hours by SEM, J/sub c/ is the highest in our studied samples. AES and TEM analyses indicate that the grain boundaries are complex multilayer structures consisting of barium-rich, copper-rich, carbon-rich, yttrium and oxygen-deficient impure phases. The dominant impure phases harmful to J/sub c/ at the boundary are the mixtures of BaCO/sub 3/, Cu/sub 2/O,BaC/sub 2/, Y/sub 2/C/sub 3/ and an amorphous material.

Research Organization:
Baoji Institute for Non-ferrous Metal Research, P.O. Box 71, Baoji, Shaanxi (CN)
OSTI ID:
5764009
Journal Information:
Int. J. Mod. Phys. B; (United States), Journal Name: Int. J. Mod. Phys. B; (United States) Vol. 3:3; ISSN IJPBE
Country of Publication:
United States
Language:
English

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