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Removal efficiency of silver impregnated filter materials and performance of iodie filters in the off-gas of the Karlsruhe reprocessing plant WAK

Conference ·
OSTI ID:567221
; ;  [1]
  1. Wiederaufarbeitungsanlage Karlsruhe (Germany); and others

An almost quantitative retention of iodine is required in reprocessing plants. For the iodine removal in the off-gas streams of a reprocessing plant various sorption materials had been tested under realistic conditions in the Karlsruhe reprocessing plant WAK in cooperation with the Karlsruhe research center FZK. The laboratory results achieved with different iodine sorption materials justified long time performance tests in the WAK Plant. Technical iodine filters and sorption materials for measurements of iodine had been tested from 1972 through 1992. This paper gives an overview over the most important results, Extended laboratory, pilot plant, hot cell and plant experiences have been performed concerning the behavior and the distribution of iodine-129 in chemical processing plants. In a conventional reprocessing plant for power reactor fuel, the bulk of iodine-129 and iodine-127 is evolved into the dissolver off-gas. The remainder is dispersed over many aqueous, organic and gaseous process and waste streams of the plant. Iodine filters with silver nitrate impregnated silica were installed in the dissolver off-gas of the Karlsruhe reprocessing plant WAK in 1975 and in two vessel vent systems in 1988. The aim of the Karlsruhe iodine research program was an almost quantitative evolution of the iodine during the dissolution process to remove as much iodine with the solid bed filters as possible. After shut down of the WAK plant in December 1990 the removal efficiency of the iodine filters at low iodine concentrations had been investigated during the following years. 12 refs., 2 figs., 2 tabs.

Research Organization:
Harvard Univ., Boston, MA (United States). Harvard Air Cleaning Lab.; USDOE Assistant Secretary for Environment, Safety, and Health, Washington, DC (United States). Office of Environmental Guidance; Nuclear Regulatory Commission, Washington, DC (United States). Office of Nuclear Regulatory Research; International Society of Nuclear Air Treatment Technologies, Inc., Batavia, OH (United States)
OSTI ID:
567221
Report Number(s):
NUREG/CP--0153; CONF-960715--; ON: TI97008959
Country of Publication:
United States
Language:
English

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