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Title: Absolute measurement of the sup 65 Cu(n,2n) sup 64 Cu, sup 64 Zn (n,p) sup 64 Cu and sup 56 Fe(n,p) sup 56 Mn cross sections at 14. 6 MeV

Thesis/Dissertation ·
OSTI ID:5665723

The {sup 65}Cu(n,2n){sup 64}Cu and {sup 64}Zn(n,p){sup 64}Cu cross sections are measured relative to the {sup 56}Fe(n,p){sup 56}Mn cross section by the activation method. The {sup 56}Fe(n,p){sup 56}Mn cross section is then measured relative to an absolutely calibrated neutron flux monitor. Neutrons are produced by a 150 kV Cockroft-Walton accelerator using the {sup 3}H(d,n){sup 4}He reaction. Measurements are conducted under low-scatter conditions at 0{degree} with respect to the incident deuteron beam direction. Measurement of the induced {sup 64}Cu activity is conducted by positron absorption and annihilation in copper. Annihilation photons are counted in two 7.6 cm {times} 7.6 cm NaI(Tl) detectors, where the counting geometry takes advantage of the angular correlation of the emitted photons. Absolute efficiency of this counting system is determined by a {sup 22}Na standard activity. The {sup 22}Na absolute source activity is determined by {beta}{sup +}-{gamma} ray coincidence counting. Induced {sup 56}Mn activity is measured by 4{kappa}{beta}{sup {minus}} counting in a gas-flow proportional counter. Absolute efficiency of this counter is determined by 4{kappa}{beta}-{gamma} coincidence counting techniques. In all measurements, the time-dependence of the neutron flux is monitored by a standard BF{sub 3} long counter in multichannel scaling mode. Absolute measurement of the neutron flux is conduced by the Dual-Thin Scintillator (DTS) detector developed at the National Bureau of Standards (NBS). Absolute efficiency of the DTS detector is measured at NBS by the time-correlated associated alpha particle technique. The calibration agrees with efficiency determined by a Monte Carlo simulation of the detector response.

Research Organization:
Michigan Univ., Ann Arbor, MI (USA)
OSTI ID:
5665723
Resource Relation:
Other Information: Thesis (Ph. D.)
Country of Publication:
United States
Language:
English

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