Estimation of cesium-137 release from waste/cement composites using data from small-scale specimens
Technical Report
·
OSTI ID:5659169
A study has been performed, correlating the leachability of Cs-137 from small-scale to large-scale waste/cement composites. In the study, simulants of two contrasting waste types were considered: cation-exchange resin and boric acid wastes incorporated in Portland Type cements. Test specimens were right cylinders of dimensions varying from 5 x 5 to 55 x 55 (diameter x height, cm). Using leach data representing diffusion-controlled release, effective diffusivities of approx. 2 x 10/sup -8/ cm/sup 2//s have been calculated for Cs-137 in both waste/cement matrices. A comparison of the observed and predicted cesium release values indicated that leach data derived from testing of small-scale specimens can be extrapolated, using a planar semi-infinite medium approximation, to estimate leachability of a full-scale specimen.
- Research Organization:
- Brookhaven National Lab., Upton, NY (USA)
- DOE Contract Number:
- AC02-76CH00016
- OSTI ID:
- 5659169
- Report Number(s):
- NUREG/CR-3382; BNL-NUREG-51690; ON: DE84002392
- Country of Publication:
- United States
- Language:
- English
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Related Subjects
052002* -- Nuclear Fuels-- Waste Disposal & Storage
12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE WASTES FROM NUCLEAR FACILITIES
36 MATERIALS SCIENCE
360604 -- Materials-- Corrosion
Erosion
& Degradation
ALKALI METAL ISOTOPES
BETA DECAY RADIOISOTOPES
BETA-MINUS DECAY RADIOISOTOPES
BORIC ACID
BUILDING MATERIALS
CEMENTS
CESIUM 137
CESIUM ISOTOPES
DATA
DISSOLUTION
EXPERIMENTAL DATA
HYDROGEN COMPOUNDS
INFORMATION
INORGANIC ACIDS
ISOTOPES
LEACHING
LOW-LEVEL RADIOACTIVE WASTES
MATERIALS
NUCLEI
NUMERICAL DATA
ODD-EVEN NUCLEI
PORTLAND CEMENT
RADIOACTIVE MATERIALS
RADIOACTIVE WASTES
RADIOISOTOPES
SEPARATION PROCESSES
SURFACE AREA
SURFACE PROPERTIES
VOLUME
WASTES
YEARS LIVING RADIOISOTOPES
12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE WASTES FROM NUCLEAR FACILITIES
36 MATERIALS SCIENCE
360604 -- Materials-- Corrosion
Erosion
& Degradation
ALKALI METAL ISOTOPES
BETA DECAY RADIOISOTOPES
BETA-MINUS DECAY RADIOISOTOPES
BORIC ACID
BUILDING MATERIALS
CEMENTS
CESIUM 137
CESIUM ISOTOPES
DATA
DISSOLUTION
EXPERIMENTAL DATA
HYDROGEN COMPOUNDS
INFORMATION
INORGANIC ACIDS
ISOTOPES
LEACHING
LOW-LEVEL RADIOACTIVE WASTES
MATERIALS
NUCLEI
NUMERICAL DATA
ODD-EVEN NUCLEI
PORTLAND CEMENT
RADIOACTIVE MATERIALS
RADIOACTIVE WASTES
RADIOISOTOPES
SEPARATION PROCESSES
SURFACE AREA
SURFACE PROPERTIES
VOLUME
WASTES
YEARS LIVING RADIOISOTOPES