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Two-dimensional intrinsic and extrinsic ferromagnetic behavior of layered La{sub 1.2}Sr{sub 1.8}Mn{sub 2}O{sub 7} single crystals

Journal Article · · Physical Review, B: Condensed Matter
; ;  [1];  [2]; ; ; ;  [3]
  1. Materials Science Division, Argonne National Laboratory, Argonne, Illinois 60439 (United States)
  2. Science and Technology Center for Superconductivity, Argonne National Laboratory, Argonne, Illinois 60439 (United States)
  3. Materials Science Division and Science and Technology Center for Superconductivity, Argonne National Laboratory, Argonne, Illinois 60439 (United States)

The low-field magnetization M and susceptibility {chi} are reported for the two-layered Ruddleson-Popper phase SrO(La{sub 1{minus}x}Sr{sub x}MnO{sub 3}){sub 2} for x=0.4 (denoted La{sub 1.2}Sr{sub 1.8}Mn{sub 2}O{sub 7}) with an in-plane magnetic easy axis. As T approaches the Curie temperature ( T{sub C}=116 K) on cooling, where the metal-insulator transition occurs in zero field, {chi} diverges as H{sup {minus}1/{delta}{sup {prime}}}, with {delta}=21{plus_minus}5. Also, near an extrinsic Curie transition attributed to {approximately}0.1{percent} volume fraction of intergrowths at T{sup {asterisk}}=2.47 T{sub C}, M scales as (1{minus}T/T){sup {beta}}, with {beta}=0.25{plus_minus}0.02. These results can be understood within the context of two-dimensional XY models, and provide some perspective of the layered manganites. {copyright} {ital 1998} {ital The American Physical Society}

OSTI ID:
565870
Journal Information:
Physical Review, B: Condensed Matter, Journal Name: Physical Review, B: Condensed Matter Journal Issue: 1 Vol. 57; ISSN 0163-1829; ISSN PRBMDO
Country of Publication:
United States
Language:
English

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