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Influence of third-harmonic fields on multiphoton ionization of noble gases in unfocused laser beams

Journal Article · · Phys. Rev. A; (United States)
Unfocused linearly polarized laser beams, in single-pass and counterpropagating configurations, are used in conjunction with absolute ionization measurements in calibrated proportional counters to examine the nature of multiphoton ionization of xenon near three-photon resonances. Mixtures of xenon with other noble gases are also used to incorporate phase matching in order to elucidate additional characteristics of multiphoton ionization in the presence of third-harmonic fields. Point-by-point comparisons are made between theoretically predicted and experimentally observed features of the study. We also show how detailed information on multiphoton ionization involving phase-matched third-harmonic photons can be used to obtain optical constants in the vacuum-ultraviolet region.
Research Organization:
Chemical Physics Section, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831
DOE Contract Number:
AC05-84OR21400
OSTI ID:
5648159
Journal Information:
Phys. Rev. A; (United States), Journal Name: Phys. Rev. A; (United States) Vol. 34:2; ISSN PLRAA
Country of Publication:
United States
Language:
English