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Excitonic optical nonlinearity induced by internal field screening in (211) oriented strained-layer superlattices

Journal Article · · Applied Physics Letters; (USA)
DOI:https://doi.org/10.1063/1.104568· OSTI ID:5636826
; ; ;  [1]; ;  [2]
  1. Los Alamos National Laboratory, Los Alamos, New Mexico 87545 (US)
  2. ECE, University of California, Santa Barbara, California 93106 (USA)
The nonlinear optical properties of a new class of strained-layer superlattices (intrinsic Stark effect superlattices) have been investigated. Specifically, we have compared the nonlinear transmission of Ga{sub 1{minus}{ital x}}In{sub {ital x}}As-GaAs strained-layer superlattices grown along the (211) axis to identical superlattices grown along the (100) axis, and found that the optical nonlinearity in the (211) sample is about one order of magnitude greater than in the (100) sample. A blue shift of the exciton resonance and an increase in the exciton absorption strength in the (211) sample with increasing light intensity was observed (attributed to screening of the intrinsic Stark effect fields by photogenerated carriers), resulting in the stronger optical nonlinearity. The maximum of the nonlinear absorption index, {vert bar}{alpha}{sub 2}{vert bar}, in the (211) sample was 54 cm/W ({vert bar}Im {chi}{sup 3}{vert bar}=0.33 esu) whereas in the (100) sample the maximum of {vert bar}{alpha}{sub 2}{vert bar} was 6.9 cm/W ({vert bar}Im {chi}{sup 3}{vert bar}=0.042 esu). The measured carrier recovery time in both samples was 2 ns.
OSTI ID:
5636826
Journal Information:
Applied Physics Letters; (USA), Journal Name: Applied Physics Letters; (USA) Vol. 58:7; ISSN APPLA; ISSN 0003-6951
Country of Publication:
United States
Language:
English

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