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U.S. Department of Energy
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Cadmium sulfide/copper ternary heterojunction cell research: Final subcontract report, 1 October 1984-31 May 1987

Technical Report ·
DOI:https://doi.org/10.2172/5626015· OSTI ID:5626015

This is the final technical progress report on a thirty-two month research program on CuInSe/sub 2/ and CuInGaSe/sub 2/ based thin-film polycrystalline heterojunction solar cells. CuInGaSe/sub 2/ films incorporating Ga fractions (x in CuIn/sub 1-x/Ga/sub x/Se/sub 2/) from 0.04 to 1.0 have been prepared and characterized. CuInGaSe/sub 2//CdZnS heterojunction devices have been fabricated for a range of Ga contents and show the expected variations in Voc and spectral response with Ga content. An efficiency of 10.2% (SERI test, ASTM87) has been measured for a cell with Ga fraction of 0.23, the highest efficiency reported for this material. A CuInSe/sub 2//CdZnS monolithically interconnected four cell series string of 91 cm/sup 2/ area has been fabricated with a total area efficiency of 9.5% (SERI test, ASTM87). Results are presented on Ion-Assisted Deposition of the selenide and sulfide, on a new design for the Se evaporation source, on ITO reactive sputter deposition, and on CdZnS films prepared from an E-Gun Evaporation source. Spectral response and I-V characteristic variations with selenide composition before and after heat-treatment are discussed for the CuInSe/sub 2//CdZnS devices. The highest AM1 total area efficiency for the CuInSe/sub 2//CdZnS cell is now 11.9% (Boeing test, AM1 spectrum) with five cells measured over the previously reported high of 10.9%. Room Temperature Photoluminescence, Voltage Contrast Imaging of junction cross sections, Raman spectroscopy, and EXAFS measurements on the CuInSe/sub 2//CdZnS devices are also presented and discussed. 45 refs., 41 figs.

Research Organization:
Boeing Co., Seattle, WA (USA). High Technology Center
DOE Contract Number:
AC02-83CH10093
OSTI ID:
5626015
Report Number(s):
SERI/STR-211-3230; ON: DE88001122
Country of Publication:
United States
Language:
English