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Measurement of Radon Diffusion from Uranium Mill Tailing Piles

Technical Report ·
DOI:https://doi.org/10.2172/5614800· OSTI ID:5614800

The concentrations of 226Ra and 222Rn (214Pb) were measured as a function of depth within a uranium mill tailings pile by in-situ gamma-ray spectrometry. Radon diffusion and exhalation rates were determined from the concentration gradients by employing an integral solution of the diffusion equation that accommodates a nonuniform depth distribution of the parent radium. Radon diffusion coefficients of 0.0002 and 0.0017 cm2/sec, and exhalation rates of 60 and 275 atoms/cm2/sec were determined for two locations with differing soil moisture content.

Research Organization:
Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)
Sponsoring Organization:
USDOE; USNRC
DOE Contract Number:
EY-76-C-06-1830
OSTI ID:
5614800
Report Number(s):
PNL--3187; NUREG/CR-1109
Country of Publication:
United States
Language:
English