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Experimental and theoretical investigations of the decays of /sup 206/Fr and /sup 208/Fr. [100 to 150 MeV]

Technical Report ·
DOI:https://doi.org/10.2172/5612055· OSTI ID:5612055
/sup 206/Fr and /sup 208/Fr were mass separated and observed with large-volume semiconductor detectors in calibrated geometries. Alpha, gamma, and electron singles and gamma-gamma and gamma-electron coincidence data were taken. The alpha decay experiments permitted the determination of the alpha branching ratios for /sup 206/ /sup 208/Fr as well as /sup 205/ /sup 207/Fr. The method used includes the information obtained from the electron capture decay studies of those nuclei. The alpha branching ratios obtained are generally higher than those reported previously. Energies and half-lives are in general agreement with previous measurements. The alpha measurements also revealed the presence of a heretofore unobserved alpha-emitting isomer in /sup 206/Fr. The isomer has a half-life of 0.7 +- 0.1 seconds, and the energy of the associated alpha decay is 6.930 +- 0.005 MeV. Gamma data taken with the alpha measurements suggest that the isomeric level is 531 keV above the /sup 206/Fr ground state, with the associated alpha decay populating a level at 391 keV in the /sup 202/At nucleus. Measured alpha branching ratios were analyzed with the Rasmussen reduced width formalism. All observed francium decays were deduced to be unhindered. This study produced detailed level schemes for /sup 206/Rn and /sup 208/Rn. The gamma and electron data permitted the determination of internal conversion coefficients, multipolarities, spins, and parities. It appears from systematics that two different bands of states above J/sup ..pi../ = 4+ are populated by in-beam studies. The deduced level scheme of /sup 208/Rn was studied in the interacting boson approximation (IBA) with the computer code PHINT. The level scheme is readily explained with this model up to around 2 MeV. Good agreement between theory and experiment was also obtained for /sup 204/Rn and /sup 206/Rn.
Research Organization:
South Carolina Univ., Columbia (USA). Dept. of Physics and Astronomy
DOE Contract Number:
EY-76-C-05-0033
OSTI ID:
5612055
Report Number(s):
DOE/TIC-11100
Country of Publication:
United States
Language:
English

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