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Thermal conductivity of Na/sub 3/(U/sub 1-y/Pu/sub y/)O/sub 4/: A preliminary in-pile determination

Conference ·
OSTI ID:5589461
During Run-Beyond-Cladding-Breach (RBCB) operation in an oxide LMR, the performance of a breached fuel element is intimately associated with the formation of fuel-sodium reaction product (FSRP), Na/sub 3/(U/sub 1-y/Pu/sub y/)O/sub 4/. In-pile experiments coupled with destructive examinations of breached fuel have consistently revealed noticeable changes in fuel structure accompanying FSRP formation at the fuel surface. Previous analyses have also indicated a significant impact of FSRP on fuel centerline temperature. Successful modeling of breached fuel thermal behavior therefore requires a reasonably accurate knowledge of the thermal properties of the FSRP, especially its thermal conductivity. But laboratory investigations have been scarce and limited to the Na/UO/sub 2/ system because of the toxicity of plutonium and hygroscopicity of the FSRP. Hence, post-irradiation observations of fuel samples remain the most amenable way of deriving the thermal conductivity of the FSRP. Such work is a spin-off of the RBCB program in the Experimental Breeder Reactor-II (EBR-II), a program jointly sponsored by the US Department of Energy and the Power Reactor and Nuclear Fuel Development Corporation of Japan.
Research Organization:
Argonne National Lab., IL (USA); Power Reactor and Nuclear Fuel Development Corp., Oarai, Ibaraki (Japan). Oarai Engineering Center
DOE Contract Number:
W-31109-ENG-38
OSTI ID:
5589461
Report Number(s):
CONF-871101-76; ON: DE88003034
Country of Publication:
United States
Language:
English