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Resonantly enhanced vacuum ultraviolet generation and multiphoton ionization in carbon monoxide gas

Journal Article · · Appl. Phys. Lett.; (United States)
DOI:https://doi.org/10.1063/1.93228· OSTI ID:5576351

Competition between three-photon resonantly enhanced vacuum ultraviolet third-harmonic generation and six-photon multiphoton ionization using the A state in gaseous carbon monoxide is observed. Excitation spectra of the third-harmonic emission exhibit increasing blue shifts and broadening with increasing pressure due to the phase matching requirements. Estimates for the efficiency and tunability show that third-harmonic generation in carbon monoxide molecules is a promising source for coherent vacuum ultraviolet light.

Research Organization:
University of California, Los Alamos National Laboratory, Los Alamos, New Mexico 87545
DOE Contract Number:
W-7405-ENG-36
OSTI ID:
5576351
Journal Information:
Appl. Phys. Lett.; (United States), Journal Name: Appl. Phys. Lett.; (United States) Vol. 40:8; ISSN APPLA
Country of Publication:
United States
Language:
English