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Sensitivities of the radiative forcing due to large loadings of smoke and dust aerosols

Journal Article · · J. Geophys. Res.; (United States)

Sensitivities of the optical properties and of the radiative perturbations induced by the microphysical characteristics of smoke and dust aerosols in the aftermath of a nuclear war are investigated. All optical calculations assume homogeneous spherical particles, prescribed by lognormal size distributions. A change in the mode radius of the aerosol size distribution between 0.1 and 1.0 ..mu..m, for a constant smoke loading, results in a tenfold decrease in the visible optical depth. Over the same size range the long-wave optical depth increases from 1/30 of the visible optical depth for a mode radius of 0.1 ..mu..m to 1/2 for a mode radius of 1.0 ..mu..m. The direct radiative forcing is studied using a spectrally dependent, one-dimensional radiative transfer model. The radiative heating is strongly influenced by the vertical distribution of smoke and dust aerosols. When compared with a constant density profile, the maximum in the heating rate, owing to a 3-km, scale height profile of smoke aerosols (visible optical depth approx.3), is reduced from 16/sup 0/ to 4/sup 0/ K/d and is more widely distributed in the troposphere. Solar absorption in the troposphere is reduced by increases in dust loadings in the stratosphere (a loading of 0.5 g/m/sup 2/ results in a 30% reduction), while the planetary albedo is enhanced over the smoke-only case (up to 150% for 0.5 g/m/sup 2/). Perturbations to the long-wave fluxes due to aerosols are modulated by the column amount of water vapor. The increase in the long-wave flux at the surface, however, even for an order of magnitude enhancement in water vapor, is less than the decrease in the solar flux.

Research Organization:
National Center for Atmospheric Research, Boulder, Colorado
OSTI ID:
5562271
Journal Information:
J. Geophys. Res.; (United States), Journal Name: J. Geophys. Res.; (United States) Vol. 90:D3; ISSN JGREA
Country of Publication:
United States
Language:
English