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Development and application of the electrochemical etching technique

Technical Report ·
OSTI ID:5561922
This report documents the advances achieved in the development and application of several etched damage track plastic dosimeters that can be used to measure dose-equivalent from neutrons with energies from thermal to 20 MeV. The project was initiated with the design of a rem-responding dosimeter that measured fast (> 1 MeV) neutron dose-equivalent as a function of the damage track density directly induced within the volume of polycarbonate foils amplified by electrochemical etching. Stillwagon (1978) adapted electrochemical etching of polycarbonate foils (ECEPF) to alpha dosimetry and used the technique to determine Pu-239 uptake in human bone. Su (1979) extended the usefulness of the ECEPF neutron dosimetry technique to encompass thermal neutron dose measurement. The thermal neutron dosimeter was composed of an external radiator tablet made of /sup 7/LiF in contact with a polycarbonate foil and utilized the thermal neutron-induced /sup 6/Li(n, ..cap alpha..)/sup 3/H reaction to give a dose-equivalent response as a function of alpha track density registered in the detector foil. An intermediate (1 eV-1 MeV) neutron dosimeter was developed and has been shown to give an approximately dose-equivalent response to neutrons with energies from 1 eV to 17 MeV. The intermediate neutron dosimeter consists of /sup 6/LiF-Teflon/CR-39 Polymer foil assembly which is enclosed by a (Cd + In) neutron filter. The neutron dose-equivalent is measured as a variable function of the damage track density registered in the CR-39 detector foil due to alpha particles from the 1/v dependent /sup 6/Li(n, ..cap alpha..)/sup 3/H reaction, recoil H, C, O nuclei from neutron-induced elastic scattering within the foil volume, and protons from the /sup 6/Li(n, p) reaction for neutron energies above 2 MeV. 46 figs., 6 tabs.
Research Organization:
Georgia Inst. of Tech., Atlanta (USA). School of Mechanical Engineering
DOE Contract Number:
AS05-76EV04814
OSTI ID:
5561922
Report Number(s):
DOE/EV/04814-T2; ON: DE85010302
Country of Publication:
United States
Language:
English