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Hexatic order in thin smectic-{ital F} liquid-crystal films

Journal Article · · Physical Review. E, Statistical Physics, Plasmas, Fluids, and Related Interdisciplinary Topics
; ; ;  [1]
  1. Department of Physics, Massachusetts Institute of Technology, Cambridge, Massachusetts 02139 (United States)

We report a synchrotron x-ray study of the stacked hexatic smectic-{ital F} phase and the smectic-{ital F} (Sm-{ital F}){r_arrow}smectic-{ital C} (Sm-{ital C}) phase transition in {similar_to}200 and {similar_to}60 molecular layer thick films of terephthal-bis-(20)-alkylanilines. A diffraction geometry is developed to facilitate the measurements on freely suspended liquid-crystal films. Deep in the hexatic Sm-{ital F} phase, both films show a high degree of orientational order. The effects of the surface ordering field in thin liquid-crystal films are discussed. In both samples, the phase transition from the Sm-{ital F} phase to the Sm-{ital C} phase is strongly first order, in contrast with the continuous Kosterlitz-Thouless hexatic-isotropic phase transition predicted for two-dimensional systems.

Research Organization:
Brookhaven National Laboratory
DOE Contract Number:
AC02-76CH00016
OSTI ID:
55237
Journal Information:
Physical Review. E, Statistical Physics, Plasmas, Fluids, and Related Interdisciplinary Topics, Journal Name: Physical Review. E, Statistical Physics, Plasmas, Fluids, and Related Interdisciplinary Topics Journal Issue: 6 Vol. 51; ISSN PLEEE8; ISSN 1063-651X
Country of Publication:
United States
Language:
English

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