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Phase equilibrium predictions for polar and hydrogen bonding mixtures

Technical Report ·
OSTI ID:5497276
The Perturbed-Hard-Chain Theory (PHCT) has been generalized to treat pure compounds and mixtures with polar forces (dipoles and quadrupoles) as well as hydrogen bonding. The generalization to polar compounds is based on the perturbation expansion for anisotropic molecules by Gubbins and coworkers. The effects of hydrogen bonding are taken into account using an approach similar to that of Heidemann and Prausnitz. With these two generalizations, accurate mixture VLE and LLE predictions can be made, even for highly non-ideal systems, using pure component parameters alone. 8 refs., 4 figs.
Research Organization:
Johns Hopkins Univ., Baltimore, MD (USA). Dept. of Chemical Engineering
DOE Contract Number:
AC02-81ER10982
OSTI ID:
5497276
Report Number(s):
DOE/ER/10982-T1; ON: DE86011812
Country of Publication:
United States
Language:
English

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