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Temperature and depth dependence of positron annihilation parameters in YBa/sub 2/Cu/sub 3/O/sub 7-. / and La/sub 1. 85/Sr/sub 0. 15/CuO/sub 4/

Conference ·
OSTI ID:5485120
The temperature dependence of the positron annihilation parameters for YBa/sub 2/Cu/sub 3/O/sub 7-x/ x = 0.7, 0.4 and 0.0 and La/sub 1.85/Sr/0.15/CuO/sub 4/ were measured. The depth dependence of the YBa/sub 2/Cu/sub 3/O/sub 7/ was studied using a variable-energy positron beam showing a strong depth dependence in the Doppler line-shape extending up to an average depth of approx.5.0 ..mu..m. It was found that a transition in the Doppler line-shape parameter, ''S'', was associated with the superconducting transition temperature (T/sub c/) in YBa/sub 2/Cu/sub 3/O/sub 7-x/ x = 0.4 and 0.0 while no transition was observed in the superconducting YBa/sub 2/Cu/sub 3/O/sub 6.3/. Positron lifetime parameters in YBa/sub 2/Cu/sub 3/O/sub 7/ were found to be consistent with positrons localized at open volume regions (probably unoccupied crystallographic sites) in this material with a lifetime of 210 psec at 300 K. These results indicate that the electron density at these unoccupied sites increases, using a free electron model, approximately 9% between 100 and 12 K. 15 refs., 4 figs.
Research Organization:
Brookhaven National Lab., Upton, NY (USA)
DOE Contract Number:
AC02-76CH00016
OSTI ID:
5485120
Report Number(s):
BNL-40445; CONF-871125-18; ON: DE88003494
Country of Publication:
United States
Language:
English

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