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Title: Studies of the single-mode and multimode cw dye lasers as sources for obtaining power-squared corrected two-photon spectra

Journal Article · · J. Appl. Phys.; (United States)
DOI:https://doi.org/10.1063/1.328015· OSTI ID:5477449

The single-mode and multimode free-running dye lasers are examined as possible sources for generating power-squared corrected two-photon absorption spectra. The observed differences between the two sources is attributed to the presence of mode noise in the multimode output, which yields inaccuracies in spectra when used as a source for two-photon spectroscopy. Using an accurate reference spectrum generated with the single-mode source, the utility of ratioing to obtain accurate spectra with the multimode laser is demonstrated. Alternate techniques for obtaining power-squared corrected two-photon spectra with the multimode laser are considered.

Research Organization:
Department of Chemistry, Purdue University, West Lafayette, Indiana 47907
OSTI ID:
5477449
Journal Information:
J. Appl. Phys.; (United States), Vol. 51:5
Country of Publication:
United States
Language:
English

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