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Significance of regional source contributions to urban PM-10 concentrations

Journal Article · · J. Air Pollut. Control Assoc.; (United States)
Based on data collected in St. Louis, Philadelphia and other eastern US cities, we conclude that a significant fraction of the PM-10 concentration is background. In these urban areas the background fraction ranges from 35 to 80 percent of the daily, monthly or annual concentration. The bulk of the background appears to be of regional origin. The average chemical makeup of eastern US PM-10 is sulfate as SO/sub 4/, 21-34 percent; crustal material, 14-39 percent; unknown (carbonaceous matter, ammonium, nitrate and water), 36-51 percent, all of which is difficult to apportion to specific sources. Dispersion modeling using a local source inventory can account only for a small portion of the total PM-10 mass. Emission roll-back of local sources may have a limited effect on reducing total concentrations of PM-10.
Research Organization:
Massachusetts Institute of Technology, Cambridge (USA)
OSTI ID:
5412876
Journal Information:
J. Air Pollut. Control Assoc.; (United States), Journal Name: J. Air Pollut. Control Assoc.; (United States) Vol. 37:11; ISSN JPCAA
Country of Publication:
United States
Language:
English