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U.S. Department of Energy
Office of Scientific and Technical Information

Coal pretreatment for two stage liquefaction. Quarterly report, April 1-June 30, 1986

Technical Report ·
OSTI ID:5402124

Efforts have been continued to examine the utility of liquid-liquid separation for the pretreatment of subbituminous coals. Reasonable separations have been obtained in terms of yield, the enrichment of reactive macerals and the rejection of mineral matter when using a coal-derived distillate as the nonaqueous medium. An investigation of the influence of reaction conditions on temperature-staged catalytic liquefaction has been continued using tubing bomb reactors. With fixed second stage conditions (425/sup 0/C, 10 min), a survey has indicated that, for a subbituminous coal, first stage reaction at 275/sup 0/C and 30 min gives good overall conversion and a high-oil to asphaltene ratio. Using these conditions for the first stage, a survey has now been started to examine the influence of the second stage conditions on the net product distribution. Preliminary results show that higher oil yields are obtained at 450 than at 425/sup 0/C without incurring excessive production of light hydrocarbon gases. Some studies have been made to examine the effect of catalyst concentration on temperature-staged liquefaction. Reducing the Mo concentration from 1.0 to 0.1% wt lowered the overall conversion by 7% and the oil yield by about 4%. The influence of solvent composition upon temperature-staged liquefaction has been studied using six distillate solvents supplied by Conoco Coal Research. Reactions were conducted in the 300 cc stirred autoclave using both subbituminous and bituminous coals. Preliminary data are presented and discussed. 5 refs., 2 figs., 8 tabs.

Research Organization:
Pennsylvania State Univ., University Park (USA). Coll. of Earth and Mineral Sciences
DOE Contract Number:
FG22-84PC70003
OSTI ID:
5402124
Report Number(s):
DOE/PC/70003-T10; ON: DE86014031
Country of Publication:
United States
Language:
English