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Structure of the major carbohydrate fragment of the Leishmania donovani lipophosphoglycan

Journal Article · · Biochemistry; (United States)
DOI:https://doi.org/10.1021/bi00393a042· OSTI ID:5400329

The major carbohydrate fragment from the lipophosphoglycan of Leishmania donovani was generated by mild acid hydrolysis (0.02 N HCl, 5 min, 100/sup 0/C) and purified by chromatography on DE-52 cellulose and thin layer. By a combination of analyses including gas-liquid chromatography-mass spectrometry and /sup 1/H NMR, the structure of the fragment was elucidated as PO/sub 4/..-->..6Gal(..beta..1-..-->..4)Man. Approximately 16 of these phosphorylated disaccharide units occur in the overall glycoconjugate structure. NMR analysis of an alkaline phosphatase treated phosphorylated tetrasaccharide generated from lipophosphoglycan showed that the phosphorylated disaccharide units are linked together via ..cap alpha..-glycosidic linkages. Complete characterization of the phosphorylated disaccharide units of lipophosphoglycan provides the first example of a defined carbohydrate anchored in membranes by a derivative of phosphatidylinositol.

Research Organization:
Univ. of Kentucky Medical Center, Lexington
OSTI ID:
5400329
Journal Information:
Biochemistry; (United States), Journal Name: Biochemistry; (United States) Vol. 26:19; ISSN BICHA
Country of Publication:
United States
Language:
English

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