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Lateral interaction energy derived from Frumkin isotherm for c(2 x 2) Br/Ag(100)

Conference ·
OSTI ID:537264
;  [1];  [2]
  1. Brookhaven National Lab., Upton, NY (United States)
  2. Univ. of Ulm (Germany). Dept. of Electrochemistry
The structure of the bromide adlayer on Ag(100) and the adsorption isotherm have been determined by using in situ surface x-ray scattering techniques and chronocoulometry. Bromide adsorbed on Ag(100) forms a fourfold-hollow-site lattice gas and the adsorption saturates at 1/2 monolayer in a c(2 x 2) structure. The Frumkin isotherm has been employed to fit the experimentally obtained isotherm. Using the experimentally determined electrosorption valency, the lateral interaction energy of 220 meV/atom at full coverage is obtained.
Research Organization:
Brookhaven National Lab., Upton, NY (United States)
Sponsoring Organization:
USDOE Office of Energy Research, Washington, DC (United States); Deutsche Forschungsgemeinschaft, Bonn (Germany); North Atlantic Treaty Organization, Brussels (Belgium)
DOE Contract Number:
AC02-76CH00016
OSTI ID:
537264
Report Number(s):
BNL--64728; CONF-970517--; ON: DE98000311
Country of Publication:
United States
Language:
English

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