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Diffusional separation of gases and solutes in oscillatory flow

Journal Article · · Separation Science and Technology; (United States)

The authors present a method for separating gases and solutes by oscillating the fluid column. The process is based on augmented diffusion and is akin to Taylor dispersion. The augmentation of the flux, as compared to simple molecular diffusion, is 3 orders of magnitude in the gaseous system and 6 orders of magnitude in the liquid system. Proper choice of experimental conditions (capillary radius, frequency, and fluid properties) is crucial for best results. In the gaseous system, the best separation factor achieved was 0.4; the expected separation under the conditions prevailing was 0.3. Highest diffusional flux was 850 m/min in a system with a cross-sectional area of 8.62 cm{sup 2}. The net energy consumption at these conditions was only 14 W. The separation in the liquid system was similar to that in the gaseous system. The method provides good separation at low energy cost.

OSTI ID:
5367526
Journal Information:
Separation Science and Technology; (United States), Journal Name: Separation Science and Technology; (United States) Vol. 26:4; ISSN SSTED; ISSN 0149-6395
Country of Publication:
United States
Language:
English

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