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Spectral output from a premixed chain reaction cw HF laser

Journal Article · · J. Appl. Phys.; (United States)
DOI:https://doi.org/10.1063/1.328191· OSTI ID:5347158
Spectral measurements of the output from a purely chemical chain reaction cw HF laser are reported. The laser is a subsonic H/sub 2/-F/sub 2/ flame, with supersonic premixing and spatially uniform initiation by a stationary normal shock. Initial chemical production of fluorine atoms is by the bimolecular reaction of F/sub 2/ with NO. Spectral measurements of the laser output near the initiating shock indicate lasing transitions in the P branches of the v=3 ..-->.. v=2, v=2 ..-->.. v=1, and v=1 ..-->.. v=0 HF bands. Further downstream, the upper vibrational levels are strongly deactivated, and lasing occurs only in the v=1 ..-->.. v=0 band. Laser emission in the v=2 ..-->.. v=1 band reappears at reduced NO flow rates, suggesting efficient deactivation of HF (v) by NO, possibly through multiquantum V-V exchange. An approximate rate of 5 x 10/sup -13plus-or-minus0.5/ cm/sup 3//sec for deactivation of HF (v=2) by NO is inferred.
Research Organization:
Center for Chemical and Environmental Physics, Aerodyne Research, Inc., Bedford Research Park, Crosby Drive, Bedford, Massachusetts 01730
OSTI ID:
5347158
Journal Information:
J. Appl. Phys.; (United States), Journal Name: J. Appl. Phys.; (United States) Vol. 51:7; ISSN JAPIA
Country of Publication:
United States
Language:
English