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Detailed investigation of the lattice structure of zeolite ZSM-11 by a combination of solid-state NMR and synchrotron X-ray diffraction techniques

Journal Article · · Journal of the American Chemical Society; (USA)
DOI:https://doi.org/10.1021/ja00189a016· OSTI ID:5300736
The lattice structure of a pure and completely siliceous sample of zeolite ZSM-11 has been investigated by a combination of high-resolution solid-state {sup 29}Si MAS NMR and synchrotron-based X-ray powder diffraction techniques. The structure is temperature dependent in the range 263-363 K and a good fit to the diffraction data at 363 K is obtained with space group I{anti 4}m2 and a{sub 0} = 20.067 (1) and c{sub 0} = 13.411 (1). At room temperature the XRD data cannot be refined as the structure is intermediate and the lattice structure of the limiting low-temperature, low-symmetry form will only be deduced from data collected at 263 K.
DOE Contract Number:
AC02-76CH00016
OSTI ID:
5300736
Journal Information:
Journal of the American Chemical Society; (USA), Journal Name: Journal of the American Chemical Society; (USA) Vol. 111:7; ISSN 0002-7863; ISSN JACSA
Country of Publication:
United States
Language:
English